You need to use the lower belt gear to line up TDC, not the pulley that has the other belts...Did I read what you wrote incorrectly (it's early, so I'm guessing I did)?
That has nothing to do with the incorrect belt angle though. Hopefully you just didn't clean the mating surfaces when you put the timing gear and pulley back on. Push cam gears back on enough? I'd go over everything again..sorry.